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Theory for diffusion-limited oscillating chemical reactions

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Bussemaker, H. J. and Brito, Ricardo (1997) Theory for diffusion-limited oscillating chemical reactions. Journal of Statistical Physics, 87 (05-jun). pp. 1165-1178. ISSN 0022-4715

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Official URL: http://link.springer.com/content/pdf/10.1007%2FBF02181278




Abstract

A kinetic description of lattice-gas automaton models for reaction-diffusion systems is presented. It provides corrections to the mean-field rate equations in the diffusion-limited regime. When applied to the two-species Maginu model, the theory gives an excellent quantitative prediction of the effect of slow diffusion on the periodic oscillations of the average concentrations in a spatially homogeneous state.


Item Type:Article
Additional Information:

© 1997 Plenum Publishing Corporation. We thank D. Dab and J. P. Boon for providing us with the table with the transition rates. R.B. acknowledges financial support from D.G.I.C.y T. (Spain), project PB94-0265.

Uncontrolled Keywords:Lattice-gas automata; Violating detailed balance
Subjects:Sciences > Physics > Thermodynamics
ID Code:21929
Deposited On:24 Jun 2013 12:36
Last Modified:24 Jul 2018 11:53

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