Publication: Nuevos complejos dipirrometénicos como plataformas versátiles para aplicaciones ópticas y/o biomédicas
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2021-04-16
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Universidad Complutense de Madrid
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Abstract
La Tesis consta de una introducción general, con un resumen de los antecedentes más relevantes relacionados con el tema, así como los objetivos planteados en este trabajo. A continuación, se recogen en tres capítulos los aspectos clave desarrollados para conseguir dichos objetivos y se completa con un capítulo de conclusiones generales, otro donde se detalla la parte experimental realizada y, finalmente, un capítulo de bibliografía. En primer lugar, se presenta a los dipirrometenos (o dipirrinas) como valiosos intermedios para la obtención de diferentes tipos de sistemas, haciendo un breve resumen de su estructura, síntesis y funcionalización. Seguidamente, se presentan los dos tipos de complejos dipirrometénicos que constituyen el objetivo principal de este trabajo. Se inicia el estudio con la síntesis de derivados de la familia de los aza-BODIPYs para su aplicación como láseres de colorante y cassettes de transferencia de energía en la zona roja del espectro. Estos compuestos presentan absorción y emisión en esta zona y se encuentran prácticamente inexplorados en las aplicaciones mencionadas...
The Thesis consists of a general introduction, which includes a summary of the most relevant background related to the subject, as well as the objectives pursued in this work. Then, the key aspects developed to achieve these goals are gathered in three chapters. Finally, the Thesis would be completed with a chapter containing the general conclusions, another chapter detailing the conducted experimental techniques and procedures and, lastly, a chapter with the bibliography. First, dipyrromethenes (or dipyrrins) would be presented as valuable intermediates for obtaining different types of systems, outlining their structure, synthesis and functionalization. Next, the two types of dipyrromethenic complexes which constitute the main objective of this work would be presented.The study begins with the synthesis of derivatives from the aza-BODIPYs family for their application as dye lasers and energy transfer cassettes in the red zone of the spectrum. These compounds present absorption and emission in this zone and practically remain unexplored in the above-mentioned applications...
The Thesis consists of a general introduction, which includes a summary of the most relevant background related to the subject, as well as the objectives pursued in this work. Then, the key aspects developed to achieve these goals are gathered in three chapters. Finally, the Thesis would be completed with a chapter containing the general conclusions, another chapter detailing the conducted experimental techniques and procedures and, lastly, a chapter with the bibliography. First, dipyrromethenes (or dipyrrins) would be presented as valuable intermediates for obtaining different types of systems, outlining their structure, synthesis and functionalization. Next, the two types of dipyrromethenic complexes which constitute the main objective of this work would be presented.The study begins with the synthesis of derivatives from the aza-BODIPYs family for their application as dye lasers and energy transfer cassettes in the red zone of the spectrum. These compounds present absorption and emission in this zone and practically remain unexplored in the above-mentioned applications...
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Tesis inédita de la Universidad Complutense de Madrid, Facultad de Ciencias Químicas, Departamento de Química Orgánica, leída el 11-12-2020